Contaminant Transport in the Soil Matrix

Research Team: Yoram Cohen (PI), Jordi Grifoll (Research Scholar), Robert van de Water (Graduate Student).

This project focuses on the development of a theoretical model for the transport of chemical contaminants in the unsaturated soil matrix under the action of rainfall, soil drying, and diurnal temperature cycling. In the first phase of the project a theoretical analysis which allows the determination of the significance of a multiphase versus a pseudo-single phase transport analysis of chemical transport was developed. A multiphase soil transport (MST) model was developed to investigate the movement of organic chemicals in the soil vadose zone. The MST model incorporates a soil moisture transport model coupled with a mass transfer model. In the MST approach climatological rainfall and soil drying data for the location of interest are used for the desired simulation period. In the first phase of the study it was found that, for the Los Angeles area, contaminant flux predictions that incorporates the effect of rainfall vary significantly throughout the year (by up to two orders of magnitude). The rate of volatilization was also found to be a function of the period during which the chemical is introduced to the soil matrix, a phenomenon which is linked to the yearly distribution of rainfall. For example, benzene which is introduced into the soil matrix in January is expected to volatilize from the soil at a rate lower by about a factor of three relative to benzene which is introduced into the soil in July.